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CH-alkylation of furan derivatives under photoinduced Pd catalysis

Igor Vyacheslavovich Lavrentev 1
Igor Vyacheslavovich Lavrentev
Konstantin Evgen'evich Shepelenko 1
Konstantin Evgen'evich Shepelenko
Irina Gennad'evna Gnatiuk 1
Irina Gennad'evna Gnatiuk
Andrey Anatol'evich Aleksandrov 1
Andrey Anatol'evich Aleksandrov
Yu Zhang 2
Yu Zhang
Viktor Mikhailovich Chernyshev 1
Viktor Mikhailovich Chernyshev
1 Platov South-Russian State Polytechnic University, Novocherkassk, Russian Federation
2 Guangzhou Institute of Energy Conversion, Chinese Academy of Sciences, Guangzhou, China
Published 2023-06-13
CommunicationVolume 33, Issue 4, 494-496
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Lavrentev I. V. et al. CH-alkylation of furan derivatives under photoinduced Pd catalysis // Mendeleev Communications. 2023. Vol. 33. No. 4. pp. 494-496.
GOST all authors (up to 50) Copy
Lavrentev I. V., Shepelenko K. E., Gnatiuk I. G., Aleksandrov A. A., Zhang Yu., Chernyshev V. M. CH-alkylation of furan derivatives under photoinduced Pd catalysis // Mendeleev Communications. 2023. Vol. 33. No. 4. pp. 494-496.
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TY - JOUR
DO - 10.1016/j.mencom.2023.06.017
UR - https://mendcomm.colab.ws/publications/10.1016/j.mencom.2023.06.017
TI - CH-alkylation of furan derivatives under photoinduced Pd catalysis
T2 - Mendeleev Communications
AU - Lavrentev, Igor Vyacheslavovich
AU - Shepelenko, Konstantin Evgen'evich
AU - Gnatiuk, Irina Gennad'evna
AU - Aleksandrov, Andrey Anatol'evich
AU - Zhang, Yu
AU - Chernyshev, Viktor Mikhailovich
PY - 2023
DA - 2023/06/13
PB - Mendeleev Communications
SP - 494-496
IS - 4
VL - 33
ER -
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@article{2023_Lavrentev,
author = {Igor Vyacheslavovich Lavrentev and Konstantin Evgen'evich Shepelenko and Irina Gennad'evna Gnatiuk and Andrey Anatol'evich Aleksandrov and Yu Zhang and Viktor Mikhailovich Chernyshev},
title = {CH-alkylation of furan derivatives under photoinduced Pd catalysis},
journal = {Mendeleev Communications},
year = {2023},
volume = {33},
publisher = {Mendeleev Communications},
month = {Jun},
url = {https://mendcomm.colab.ws/publications/10.1016/j.mencom.2023.06.017},
number = {4},
pages = {494--496},
doi = {10.1016/j.mencom.2023.06.017}
}
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Lavrentev, Igor Vyacheslavovich, et al. “CH-alkylation of furan derivatives under photoinduced Pd catalysis.” Mendeleev Communications, vol. 33, no. 4, Jun. 2023, pp. 494-496. https://mendcomm.colab.ws/publications/10.1016/j.mencom.2023.06.017.

Keywords

2-hetarylfurans.
CH-alkylation
furan
palladium
photoinduced metal catalysis

Abstract

A new method for selective C(5)-H alkylation of 2-substituted furans with tertiary and secondary alkyl bromides under photoinduced by visible light (∼460 nm) palladium catalysis has been developed. The method is relied on the use of available Pd(PPh3)4 catalyst under mild conditions (30 ± 5 °C, K2CO3 as base), tolerates to various functional groups in furanic substrates and provides from good to excellent yields of alkylated products.

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